Thieves damaged three doors as they tried to break into the Falls of Shin Visitor Centre.
The incident occurred something between 8.30pm on Friday and 8.30am on Saturday.
Police said while there was damage, the culprit or culprits did not manage to enter the building and nothing was stolen.
Constable Angus Morrison said: “Our inquiries are ongoing and I would urge anyone who saw something they believe to be suspicious around that area to pass this information on as soon as possible.
“You can contact police on 101, quoting NE14337/17, or call Crimestoppers on 0800 555 111.”
Police investigate attempted break-in at north visitor centre